The Hollywood couple, who tied the knot in France in August, are going retro for By The Sea, their first film together in 10 years after Mr and Mrs Smith.
New snaps show Brad and his wife in an emotional embrace as they get into character and look incredibly different dressed up for the film.
Ang, 39, donned a blonde wig and gorgeous vintage white dress and mustard scarf, while Brad, 50, wore a cream fedora, white unbuttoned shirt and chinos.
More pictures below
Girl Interrupted star Ang, who wrote the film and is also directing, was seen chatting to crew and setting up shots as Brad also followed his wife's instructions.
Meanwhile, the Fury star was recently left red-faced after his awkward joke interview with Hangover star and now-legend Zach Galifianakis, in which he teased him about his ex-wife, Jennifer Aniston.
"Tell me what was it like when you first laid eyes on Angelina," he asked. "Was it like one of those classical love stories, like when Ross first saw Rachel? You know that show Friends, have you seen that?"
Brad looked uncomfortable but grinned and was a good sport, we imagine Ang didn't mind too much either.
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